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By completing Story Mode you will already have Agent Coulson unlocked and Lola is unlocked by completing the corresponding race in Manhattan, you will then need to purchase her. The easier way to get this is to start Agent Coulson's quest in Manhattan, he will ask you to gas up Lola for his trip. Switch to Agent Coulson and hop in the car and the trophy will unlock. If you forget to do it during the mission then you can simply wait until you unlock Lola and summon her from one of the vehicle spawn points scattered around Manhattan. The blue vehicle spawn points don't seem to allow you to spawn her so you will have to do it from a red one, the most convenient one is located on the dock underneath the Brooklyn Bridge.

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