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Gamerscore: 30G
Achievement Description: Finish Story Mode on Golden Bullets difficulty.

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You will also need to complete the game at least once on any difficulty. This will be another full play through of the game but using "Golden Bullets" which kill the enemy in one shot rather than several.

Just work your way through the story again, take your time and watch out for where all your enemies are on the screen. As you have already played through once you should have a rough idea of where most enemies are in the levels. Keep using slowmo and don't stop. The more you keep moving the less damage you will take to your health.